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Natural Analogs and Performance Assessment for Geologic Disposal of Nuclear Waste

Published online by Cambridge University Press:  10 February 2011

William M. Murphy*
Affiliation:
Center for Nuclear Waste Regulatory Analyses, Southwest Research Institute, San Antonio, TX 78228-0510USA
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Abstract

The use of natural analog studies in performance assessments has been widely discussed and debated, but its accomplishment has been limited. Given recognized uncertainties and challenges, scientific contributions to performance assessments and support for the validity of performance assessment models are valuable from all possible sources, including natural analog studies. The conceptual basis for geologic disposal of nuclear waste and for performance assessments relies on scientific expertise based largely on studies of natural systems analogous to possible repository systems, i.e., natural analogs. Natural analog studies offer contributions to model validation based both on inductive and deductive reasoning. The utility of analog studies as a deductive tool in performance assessment is enhanced by specificity of the analog system to the repository system. As geologic sites are selected and repository designs detailed, the use of analog data in supporting deductive performance assessments should increase. Consideration of Yucca Mountain for the proposed US high level nuclear waste repository affords site specificity conducive to applications of natural analog data in performance assessment. The primary use of Peñia Blanca natural analog data in recent Yucca Mountain performance assessments stems from observations of mineral products formed by alteration of natural uraninite, an analog of spent fuel. Alternate performance assessment source term models based on the Peñia Blanca oxidation rate model and the schoepite solubility model yield lower, yet comparable estimated doses than the base case model in the NRC performance assessment for Yucca Mountain.

Type
Research Article
Copyright
Copyright © Materials Research Society 2000

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References

REFERENCES

[1] Ewing, R.C., in Scientific Basis for Nuclear Waste Management (Mater. Res. Soc. Proc. 1, Pittsburgh, PA, 1979) 5768.Google Scholar
[2] Grambow, B., Jercinovic, M.J., Ewing, R.C., and Byers, C.D., in Scientific Basis for Nuclear Waste Management (Mater. Res. Soc. Proc. 50, Pittsburgh, PA, 1985) pp. 263272.Google Scholar
[3] Lutze, W., Malow, G., Ewing, R.C., Jercinovic, M.J., and Keil, K., Nature 314, 252 (1985).Google Scholar
[4] Ewing, R.C., Chakoumakos, B.C., Lumpkin, G.R., Murakami, T., Greegor, R.B., and Lytle, F.W., Nucl. Instru. Meth. Phys. Res. B32, 487 (1988).Google Scholar
[5] Finch, R.J. and Ewing, R.C., Radiochim. Acta 52/53 395 (1991).Google Scholar
[6] Janeczek, J. and Ewing, R.C., in Scientific Basis for Nuclear Waste Management (Mater. Res. Soc. Proc. 257, Pittsburgh, PA, 1992) pp. 497504.Google Scholar
[7] Pearcy, E.C., Prikryl, J.D., Murphy, W.M., and Leslie, B.W., Appl. Geochem. 9 713 (1994).Google Scholar
[8] Winograd, I.J., USGS Open-File Report 86–136 (1986).Google Scholar
[9] Neretnieks, I., in Natural Analogue Working Group First Meeting, Brussels, November 1985, edited by Côme, B. and Chapman, N.A. (CEC Nucl. Sci. Tech. EUR 10361, 1986) pp. 3236.Google Scholar
[10] Miller, W., Alexander, R., Chapman, N., McKinley, I., and Smellie, J., Natural Analogue Studies in the Geological Disposal of Radioactive Wastes (Elsevier, Amsterdam, 1994) 395 pp.Google Scholar
[11] Levy, S., in Scientific Basis for Nuclear Waste Management VII, edited by McVay, G.L. (Mater. Res. Soc. Proc., Pittsburgh, PA, 1984) 959966.Google Scholar
[12] Khoury, H.N., Salameh, E., Clark, I.P., Fritz, P., Milodowski, A.E., Cave, M.R., Bajjali, W., and Alexander, W.R., J. Geochem. Explor. 46 117 (1992).Google Scholar
[13] Matyskiela, W., Geology 25 1115 (1997).Google Scholar
[14] Ildefonse, P., Muller, J.-P., Clozel, B., and Calas, G., Engin. Geol. 29 413 (1990).Google Scholar
[15] Suksi, J., Ruskeeniemi, T., Lindberg, A., and Jaakkola, T., Radiochim. Acta 52/53 367 (1991).Google Scholar
[16] Pearcy, E.C., Prikryl, J.D., and Leslie, B.W., Appl. Geochem. 10 685 (1995).Google Scholar
[17] Smellie, J.A.T. and Karlsson, F., Engin. Geol. 53 193 (1999).Google Scholar
[18] Jarzemba, M.S., Nucl. Tech. 118 132 (1997).Google Scholar
[19] Eisenberg, N.A., Chem. Geol. 55 189 (1986).Google Scholar
[20] Sagar, B. and Wittmeyer, G.W., in Workshop on the Role of Natural Analogs in Geologic Disposal of High-Level Nuclear Waste, edited by Kovach, L.A. and Murphy, W.M. (Nuclear Regulatory Commission, NUREG/CP-0147, Washington, DC, 1995) pp. 2128.Google Scholar
[21] Alexander, W.R. and McKinley, I.G., in Proceedings of the Fourth Natural Analogue Working Group Meeting, edited by Côme, B. and Chapman, N.A. (CEC EUR 10314, 1991) pp. 119151.Google Scholar
[22] Hatch, L., Amer. Sci. 41 410 (1953).Google Scholar
[23] National Academy of Sciences, The Disposal of Radioactive Waste on Land(NAS-NRC Pub. 519, Washington, DC, 1957).Google Scholar
[24] Birchard, G.F. and Alexander, D.H., in Scientific Basis for Nuclear Waste Management (Mater. Res. Soc. Proc. 15, Pittsburgh, PA, 1983) pp. 323329.Google Scholar
[25] Crisman, D.P. and Jacobs, G.K., Native Copper Deposits of the Portage Lake Volcanics, Michigan: Their Implication with Respect to Canister Stability for Nuclear Waste Isolation in the Columbia River Basalts Beneath the Hanford Site, Washington (Rockwell International, Hanford, WA, RHOBW-ST-26 P, 1982).Google Scholar
[26] Code of Federal Regulations 10, Part 60, US Government Printing Office, Washington, DC (1998).Google Scholar
[27] Nuclear Regulatory Commission 10 CFR Part 19 et al. Federal Register 64, #34, 86408679 (1999).Google Scholar
[28] Ewing, R.C. and Jercinovic, M.J., in Scientific Basis for Nuclear Waste Management X, edited by Bates, J.K. and Seefeldt, W.B. (Mater. Res. Soc. Proc. 84, Pittsburgh, PA, 1987) pp. 6783.Google Scholar
[29] Pearcy, E.C. and Murphy, W.M., Geochemical Natural Analogs Literature Review (Center for Nuclear Waste Regulatory Analyses, CNWRA 90-008, San Antonio, TX, 1991).Google Scholar
[30] Petit, J.-C., Le Stockage des Déchets Radioactifs: Perspective Historique et Analyse Sociotechnique, Doctoral Thesis, Ecole Nationale Supédrieure des Mines de Paris, 1993.Google Scholar
[31] Oversby, V.M., in Scientific Basis for Nuclear Waste Management XXIII (Mater. Res. Soc. Proc.,2000) this volume.Google Scholar
[32] Bruno, J., Cross, J.E., Eikenberg, J., McKinley, I.G., Read, D., Sandino, A., and Sellin, P., Testing of Geochemical Models in the Poços de Caldas Analogue Study (SKB Technical Report TR 90-20 SKB, Stockholm, 1990).Google Scholar
[33] Condit, C.D. and Connor, C.B., GSA Bull. 108 1225 (1996).Google Scholar
[34] Connor, C.B. and Conway, F.M., in Encyclopedia of Volcanoes (Academic Press, 2000) pp. 381393.Google Scholar
[35] Connor, C.B. and Hill, B.E., J. Geophys. Res. 100(B6), 10,107 (1995).Google Scholar
[36] Hill, B.E., Connor, C.B., Jarzemba, M.S., Femina, P.C. La, Navarro, M., and Strauch, W., GSA Bull. 110 1231 (1998).Google Scholar
[37] McKinley, I.G., in Risk Analysis in Nuclear Waste Management, edited by Saltelli, A. et al. (ECSC, EEC, EAEC, Brussels, 1989) pp. 359396.Google Scholar
[38] Browning, L., Murphy, W.M., Leslie, B.W., and Dam, W.L., in Scientific Basis for Nuclear Waste Management XXIII (Mater. Res. Soc. Proc., 2000) this volume.Google Scholar
[39] Murphy, W.M., Pearcy, E.C., and Goodell, P.C., in Fourth Natural Analogue Working Group Meeting and Poços de Caldas Project Final Workshop, edited by Côme, B. and Chapman, N.A. (Commission of European Communities, EUR 13014 EN, 1991), pp. 267276.Google Scholar
[40] Murphy, W.M. and Pearcy, E.C., in Scientific Basis for Nuclear Waste Management XV, edited by Sombret, C. (Mater. Res. Soc. Proc. 257, 1992) pp. 521527.Google Scholar
[41] Murphy, W.M. and Codell, R.B., in Scientific Basis for Nuclear Waste Management XXII, edited by Wronkiewicz, D.J. and Lee, J.H. (Mater. Res. Soc. Proc. 556, Warrendale, PA, 1999) pp. 551558.Google Scholar
[42] Muller, J.-P., Clozel, B., Ildefonse, P., and Calas, G., Appl. Geochem. Sup. Issue 1 205 (1992).Google Scholar
[43] Prikryl, J.D., Pickett, D.A., Murphy, W.M., and Pearcy, E.C., J. Contam. Hydro. 26 61 (1997).Google Scholar
[44] Pickett, D.A. and Murphy, W.M., in Seventh EC Natural Analogue Working Group Meeting, edited by Maravic, H. von and Smellie, J. (European Commission, EUR 17851 EN, 1997) pp. 113122.Google Scholar
[45] Department of Energy, Viability Assessment of a Repository at Yucca Mountain Total System Performance Assessment (DOE/RW-0508, v. 3, Department of Energy, Las Vegas, NV, 1998).Google Scholar
[46] TRW, Total System Performance Assessment - Viability Assessment (TSPA-VA) Analyses Technical Basis Document (TRW Environmental Safety Systems Inc., Las Vegas, NV, B00000000-01717-4301-00004 Rev. 01, 1998).Google Scholar
[47] CNWRA, Total-system Performance Assessment (TPA) Version 3.2 Code: Module Descriptions and User's Guide, 1998.Google Scholar
[48] Nuclear Regulatory Commission, NRC Sensitivity and Uncertainty Analyses for a Proposed HLW Repository at Yucca Mountain, Nevada, Using TPA 3.1 Volume 1: Conceptual Models and Data, (NUREG-1668, 1, 1999).Google Scholar
[49] Nuclear Regulatory Commission, NRC Sensitivity and Uncertainty Analyses for a Proposed HLW Repository at Yucca Mountain, Nevada, Using TPA 3.1 Results and Conclusions (NUREG-1668, 2, 1999).Google Scholar
[50] Electric Power Research Institute, Alternative Approaches to Assessing the Performance and Suitability of Yucca Mountain for Spent Fuel Disposal (TR-108732, EPRI, Palo Alto, CA, 1998).Google Scholar
[51] Murphy, W.M. and Pearcy, E.C., in Fifth CEC Natural Analogue Working Group Meeting and Alligator Rivers Analogue Project (ARAP) Final Workshop, edited by Maravic, H. von and Smellie, J. (Commission of the European Communities, EUR 15176 EN, 1994) pp. 219224.Google Scholar
[52] Leslie, B.W., Pearcy, E.C., and Prikryl, J.D., in Scientific Basis for Nuclear Waste Management XVI, edited by Interrante, C.G. and Pabalan, R.T. (Mater. Res. Soc. Proc. 294, Pittsburgh, PA, 1993) pp. 505512.Google Scholar
[53] Wronkiewicz, D.J. and Buck, E.C., in Uranium: Mineralogy, Geochemistry and the Environment, edited by Burns, P.C. and Finch, R. (Min. Soc. Am. Rev. Min. 38, 1999) pp. 475497.Google Scholar
[54] Burns, P.C., Ewing, R.C., and Miller, M.L., J. Nucl. Mater. 245 1 (1997).Google Scholar
[55] Buck, E.C., Finch, R.J., Finn, P.A., and Bates, J.K., in Scientific Basis for Nuclear Waste Management XXI edited by McKinley, I.G. and McCombie, C. (Mater. Res. Soc. Proc. 506, Warrendale, PA, 1998) pp. 8794.Google Scholar
[56] Wilson, M.L. et al. Total-System Performance Assessment for Yucca Mountain - SNL Second Iteration (TSPA - 1993) (Sandia National Laboratories, SAND93-2675, 1994).Google Scholar
[57] TRW, Total System Performance Assessment - 1995: An Evaluation of the Potential Yucca Mountain Repository (TRW Environmental Safety Systems Inc., Las Vegas, NV. B00000000-01717-2200-00136, Rev. 01, 1995).Google Scholar
[58] Murphy, W.M., in Scientific Basis for Nuclear Waste Management XX, edited by Gray, W.J. and Triay, I.R. (Mater. Res. Soc. Proc. 465, Pittsburgh, PA, 1997) pp. 713720.Google Scholar
[59] Murphy, W.M., Pearcy, E.C., and Pickett, D.A., in Seventh EC Natural Analogue Working Group Meeting, edited by Maravic, H. von and Smellie, J. (European Commission EUR 17851 EN, 1997) pp. 105112.Google Scholar
[60] Murphy, W.M., Pickett, D.A., and Pearcy, E.C., in 8th EC Natural Analogue Working Group Meeting, edited by Maravic, H. von and Smellie, J. (European Commission, 2000) in press.Google Scholar
[61] Baca, R.G. and Jarzemba, M.S. (editors) Detailed Review of Selected Aspects of Total System Performance Assessment - 1995. CNWRA Letter Report to NRC, 1997.Google Scholar
[62] Hardin, E.L., Near Field/Altered Zone Models Report (Lawrence Livermore National Laboratory, Livermore, CA, UCRL-ID-129179, 1998).Google Scholar
[63] Hsi, C.-K.D. and Langmuir, D., Geochim. Cosmochim. Acta 49 1931 (1985).Google Scholar
[64] Murrell, M.T., Goldstein, S.J., and Dixon, P.R., in 8th EC Natural Analogue Working Group Meeting, edited by Maravic, H. von and Smellie, J. (European Commission, 2000) in press.Google Scholar