Hostname: page-component-78c5997874-mlc7c Total loading time: 0 Render date: 2024-11-18T10:50:11.316Z Has data issue: false hasContentIssue false

A Comprehensive Study of the 14C Source Term in the 10 MW High-Temperature Gas-Cooled Reactor

Published online by Cambridge University Press:  24 June 2019

X Liu
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
W Peng
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
L Wei
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
M Lou
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
F Xie*
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
J Cao
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
J Tong
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
F Li
Affiliation:
Institute of Nuclear and New Energy Technology, Collaborative Innovation Center of Advanced Nuclear Energy Technology, Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education, Tsinghua University, Beijing 100084, China
G Zheng
Affiliation:
Massachusetts Institute of Technology, Nuclear Reactor Laboratory, Cambridge, MA 02139, USA
*
*Corresponding author. Email: fxie@tsinghua.edu.cn.

Abstract

While assessing the environmental impact of nuclear power plants, researchers have focused their attention on radiocarbon (14C) owing to its high mobility in the environment and important radiological impact on human beings. The 10 MW high-temperature gas-cooled reactor (HTR-10) is the first pebble-bed gas-cooled test reactor in China that adopted helium as primary coolant and graphite spheres containing tristructural-isotropic (TRISO) coated particles as fuel elements. A series of experiments on the 14C source terms in HTR-10 was conducted: (1) measurement of the specific activity and distribution of typical nuclides in the irradiated graphite spheres from the core, (2) measurement of the activity concentration of 14C in the primary coolant, and (3) measurement of the amount of 14C discharged in the effluent from the stack. All experimental data on 14C available for HTR-10 were summarized and analyzed using theoretical calculations. A sensitivity study on the total porosity, open porosity, and percentage of closed pores that became open after irradiating the matrix graphite was performed to illustrate their effects on the activity concentration of 14C in the primary coolant and activity amount of 14C in various deduction routes.

Type
Conference Paper
Copyright
© 2019 by the Arizona Board of Regents on behalf of the University of Arizona 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

Footnotes

Selected Papers from the 23rd International Radiocarbon Conference, Trondheim, Norway, 17–22 June, 2018

References

REFERENCES

Brooks, LH, Heath, CA, Kirstein, B, Roberts, DG. 1974. Carbon-14 in the HTGR fuel cycle. Report No. GA-A 13174 UC-77, General Atomics, San Diego.CrossRefGoogle Scholar
Davis, W Jr. 1977. Carbon-14 production in nuclear reactors. ORNL/NUREG/TM-12, Oak Ridge National Laboratory.CrossRefGoogle Scholar
Dubourg, M. 1997. The carbon 14 cycle. Report, Le Mesnil Saint Denis, France.Google Scholar
Dunzik-Gougar, ML, Smith, TE. 2014. Removal of carbon-14 from irradiated graphite. Journal of Nuclear Materials 451:328335.CrossRefGoogle Scholar
Fachinger, J, Den Exter, M, Grambow, B, Holgersson, S, Landesman, C, Titov, M, Podruhzina, T. 2006. Behaviour of spent HTR fuel elements in aquatic phases of repository host rock formations. Nuclear Engineering and Design 236:543554.10.1016/j.nucengdes.2005.11.023CrossRefGoogle Scholar
Fachinger, J, Lensa, W, Podruhzina, T. 2008. Decontamination of nuclear graphite. Nuclear Engineering and Design 238:30863091.CrossRefGoogle Scholar
Frolov, A. 2002. Carbon-14 in gas-aerosol release from NPP with WWER type reactor. Topical report, SPAEP.Google Scholar
Haag, GL. 1991. Removal of carbon-14. In: Goossens, WRA, Eichholz, GG, Tedder, DW, editors. Radioactive waste management handbook. Vol. 2. Treatment of gaseous effluents at nuclear facilities. New York: Harwood Academic.Google Scholar
Hoinkis, E, Eatherly, WP, Krautwasser, P, Robens, E. 1986. Corrosion- and irradiation-induced porosity changes of a nuclear graphitic material. Journal of Nuclear Materials 141–143(1):8795.10.1016/S0022-3115(86)80015-0CrossRefGoogle Scholar
Hou, X. 2018. Tritium and 14C in the environment and nuclear facilities: sources and analytical methods. Journal of the Korean Radioactive Waste Society 16(1):1139.10.7733/jnfcwt.2018.16.1.11CrossRefGoogle Scholar
International Atomic Energy Agency (IAEA). 2004. Management of waste containing tritium and carbon-14. Technical Reports Series no. 421. Vienna.Google Scholar
Li, H, Liu, X, Xie, F, Jia, F. 2017. Experimental study on the content and distribution of key nuclides in an irradiated graphite sphere of HTR-10. Nuclear Engineering and Design 323:3945.CrossRefGoogle Scholar
Liu, X, Huang, X, Xie, F, Jia, F, Feng, X, Li, H. 2017. Source term analysis of irradiated graphite in the core of HTR-10. Science and Technology and Nuclear Installations 2017:2614890 (1–6).CrossRefGoogle Scholar
Liu, Z. 2004. Estimate of annual yields of 14C and 3H produced in Taiwan NPP. Radiation Protection Bulletin 141, 24(3):2326.Google Scholar
Marsden, BJ, Hopkinson, KL, Wickham, AJ. 2002. The chemical form of carbon-14 within graphite. Report No. SA/RJCB/RD03612001/R01. Issue 4. Serco Assurance.Google Scholar
McDermott, L, Jones, AN, Marsden, BJ, Marrow, TJ, Wickham, AJ. The location of radioisotopes in British experimental pile grade zero graphite waste. Conference of securing the safe performance of graphite reactor cores, Nottingham, UK, 2008, 24–26, November.Google Scholar
Nuclear Decommissioning Authority (NDA), 2012. Geological disposal carbon-14 project- Phase 1 report. NDA Report no. NDA/RWMD/092. ISBN 978-1-84029-476-7.Google Scholar
Shiozawa, S, Fujikawa, S, Iyoku, T, Kunitomi, K, Tachibana, Y. 2004. Overview of HTTR design features. Nuclear Engineering and Design 233:1121.CrossRefGoogle Scholar
Smith, TE, Mccrory, S, Dunzik-Gougar, ML. 2013. Limited oxidation of irradiated graphite waste to remove surface carbon-14. Nuclear Engineering and Technology 45(2):211218.10.5516/NET.06.2012.025CrossRefGoogle Scholar
U.S. DOE Nuclear Energy Research Advisory Committee (NERAC) and the Generation IV International Forum (GIF). 2002. A Technology Roadmap for Generation IV Nuclear Energy Systems. GIF-002-00.Google Scholar
Val’skii, G. 1976. Yields of light nuclei in ternary fission. Soviet Journal of Nuclear Physics 24(2):140144.Google Scholar
Vorobyov, A, Seleverstov, D, Grachov, V, Kondurov, I, Nikitin, A, Smirnov, N, Zalite, Yu. 1972. Light nuclei from 235U neutron fission. Physics Letters 40B(1):102104.CrossRefGoogle Scholar
Wei, L, Ma, T, Zhang, Y, Xie, F, Liu, L, Fang, X, Li, C, Xia, B, Cao, J, Chen, X. 2018. Study of an identification method of the temperature measuring pebbles in the transition core of HTR-10. Proceedings of HTR 2018. Warsaw, Poland.Google Scholar
Wenzel, U, Herz, D, Schmidt, P. 1979. Determination of 14C in spent HTGR fuel elements. Journal of Radioanalytical Chemistry 53(1–2):715.CrossRefGoogle Scholar
Xie, F, Cao, J, Feng, X, Liu, X, Tong, J, Wang, H, Dong, Y, Zhang, Z, Loyalka, SK. 2017. Experimental research on the radioactive dust in the primary loop of HTR-10. Nuclear Engineering and Design 324:372378.10.1016/j.nucengdes.2017.09.015CrossRefGoogle Scholar
Xie, F, Cao, J, Feng, X, Tong, J, Dong, Y, Zhang, Z, Scarlat, RO. 2018a. Study of tritium in the primary loop of HTR-10: Experiment and theoretical calculations. Progress in Nuclear Energy 105:99105.CrossRefGoogle Scholar
Xie, F, Li, H, Liu, X, Chen, J, Li, C, Chen, X, Verfondern, K. 2018b. A comprehensive study on source terms in irradiated graphite spheres of HTR-10. Annals of Nuclear Energy 122:352365.CrossRefGoogle Scholar
Xie, F, Peng, W, Cao, J, Feng, X, Wei, L, Tong, J, Li, F, Sun, K. 2019. Experimental investigation of 14C in the primary coolant of the 10 MW high temperature gas-cooled reactor. Radiocarbon 61(3):867884.10.1017/RDC.2019.6CrossRefGoogle Scholar
Xu, Y, Zuo, K. 2002. Overview of the 10 MW high temperature gas cooled reactor-test module project. Nuclear Engineering and Design 218:1323.10.1016/S0029-5493(02)00181-4CrossRefGoogle Scholar
Yim, M-S, Caron, F. 2006. Life cycle and management of carbon-14 from nuclear power generation. Progress in Nuclear Energy 48:236.10.1016/j.pnucene.2005.04.002CrossRefGoogle Scholar
Zhang, Z, Dong, Y, Li, F, Zhang, Z, Wang, H, Huang, X, Li, H, Liu, B, Wu, X, Wang, H, Diao, X, Zhang, H, Wang, J. 2016. The Shandong Shidao Bay 200 MWe high-temperature gas-cooled reactor pebble-bed module (HTR-PM) demonstration power plant: an engineering and technological innovation. Engineering 2:112118.10.1016/J.ENG.2016.01.020CrossRefGoogle Scholar
Zhang, Z, Wu, Z, Wang, D, Xu, Y, Sun, Y, Li, F, Dong, Y. 2009. Current status and technical description of Chinese 2×250MWth HTR-PM demonstration plant. Nuclear Engineering and Design 239:12121219.CrossRefGoogle Scholar
Zheng, G, Xu, P, Sridharan, K, Allen, T. 2011. Pore structure analysis of nuclear graphites IG-110 and NBG-18. Advances in Materials Science for Environmental and Nuclear Technology II 227:251260.Google Scholar