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Studies on the influence of structure units on the state of ytterbium ions in TeO2-based glasses

Published online by Cambridge University Press:  14 February 2020

Yonggang Liu ,
Zhongyuan Lu ,
Jianjie Xu  and
Tengxiao Guo
Yonggang Liu*
Affiliation:
Analytical and Testing Center, Southwest University of Science and Technology, Mianyang 621010, China; and Research Center of Laser Fusion, China Academy of Engineering Physics, Mianyang 621900, China
Zhongyuan Lu*
Affiliation:
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang 621010, China
Jianjie Xu
Affiliation:
State Key Laboratory of NBC Protection for Civilian, Beijing 102205, China
Tengxiao Guo
Affiliation:
State Key Laboratory of NBC Protection for Civilian, Beijing 102205, China
*
a)Address all correspondence to these authors. e-mail: s044154lyg@gmail.com
b)e-mail: Luy@swust.edu.cn
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Abstract

A simple composition of TeO2–Yb2O3 binary glass was selected as the host glass matrix for discussing the structure of tellurite glass with increasing Yb2O3 content. Raman spectra were measured to investigate the structure of the binary tellurite glasses, and upconversion and downconversion fluorescence characteristics were employed for discussing the relationship between the structural units and the state of Yb3+ in the tellurite glasses. The results suggested that the decrease of TeO4/2 in the glasses would result in the formation of Yb3+ clusters and Yb3+–O2− couple in the tellurite glasses, and then results in the decrease of cooperative upconversion and downconversion fluorescence intensity.

Keywords

Raman scatteringfluorescenceYb3+-doped tellurite glasses
Type
Article
Information
Journal of Materials Research , Volume 35 , Issue 4 , 28 February 2020 , pp. 422 - 429
Copyright
Copyright © Materials Research Society 2020

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