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Published online by Cambridge University Press: 15 February 2011
We reported a scanning tunneling microscopy(STM) observation on the growth mode transition from 2D-nucleation to spiral growth in the epitaxial Fe films on MgO(001). As the growth temperature is increased to above 493 K, a temperature region where the Schwoebel barrier is overcome, the Fe films grow in a 2D-nucleation and growth mode formed atomically flat films. The 2D-nucleation transformed into a spiral growth as increasing film thickness. At a growth temperature of 493 K, the transition of 2D nucleation to the spiral growth was observed at a film thickness of 75 Å. The critical thickness of the emergence of growth transition decreased as the growth temperature is increased.